Download e-book for iPad: Encyclopedia of Electrochemistry, Interfacial Kinetics and by Allen J. Bard, Martin Stratmann, Ernesto J. Calvo

By Allen J. Bard, Martin Stratmann, Ernesto J. Calvo

Unrivalled in its breadth and intensity, this 11-volume encyclopedia offers either a simple creation to all subject matters concerning glossy electrochemistry in addition to a accomplished assessment of the topic. all through, the emphasis is in quick access to info, with each subject taken care of at an introductory, medium and complex point. This first class reference paintings is edited and written by way of popular scientists, protecting every thing from basic learn to parts of program. Alan Bard, skilled editor of the magazine of the yankee Chemical Society, is among the most famed specialists in electrochemistry and one of many editors-in-chief.

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Equations (6) and (9) predict rate constants with a transfer coefficient of 1/2 for small overpotentials, and a constant rate klim for high overpotentials (see Fig. 2). From the form of the current-potential curve, it is clear that the Marcus-inverted region cannot be accessed in a simple redox reaction on a metal electrode. For large overpotentials, the electrons are simply transferred to energy levels above the Fermi level so that the inverted part of the energy-resolved rate plays no role. 2 η [V] Logarithm of the normalized rate constant kred /klim vs.

The latter type of processes has drawn particular attention in recent years owing to the growing interest in conduction properties of individual molecules and of molecular assemblies. 3 Electronic Tunnel Factors in Molecular Electron Transfer and Molecular Conduction {n} (a) D Θ A {l} {n} {r} (b) Θ Fig. 2 A schematic view of the electronic and nuclear states involved in typical electron transmission systems. See text for details. of intensive research owing to recent interest in electron transfer phenomena underlying the operation of the STM on one hand, and in the transmission properties of molecular bridges between conducting leads on the other.

12. W. Schmickler, J. Electroanal. Chem. 1986, 204, 31. 13. A. J. Legget, S. Chakravarty, A. T. , Rev. Mod. Phys. 1987, 59, 1. 14. D. M. Newns, Phys. Rev. 1969, 178, 1123. 15. P. P. Schmidt, Specialist Periodical Reports, Electrochemistry, The Chemical Society, London, 1975, Vol. 5, pp. 21–131. 16. S. -P. Hsu, J. Chem. Phys. 1999, 111, 11 117. 17. W. Schmickler, Chem. Phys. Lett. 1995, 237, 152. 18. W. Schmickler, Electrochim. Acta 1996, 41, 2329. 19. H. Sumi, R. Marcus, J. Chem. Phys. 1986, 84, 4894.

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